Soft Matter Soft Matter


Soft Matter

1. Bio-polymer Network Theory
Semiflexible filament networks are common in bio-systems, existing as cytoskeleton, extracellular matrix, connective tissues, etc. These filament networks exhibit unique mechanic properties compared with flexible polymer networks such as rubbers. We try to develop continuum theories to understand the complex viscoelastic properties of both permanently and transiently crosslinked filament networks. 
  • F. Meng, and E. Terentjev*, "Fluidisation of transient filament networks." Macromolecules 51, 4660–4669 (2018). 
  • F. Meng, and E. Terentjev*, "Theory of semiflexible filaments and networks." Polymers 9, 52 (2017). 
  • F. Meng, and E. Terentjev*, "Nonlinear elasticity of semiflexible filament networks." Soft Matter 12, 6749-6756 (2016). 
2. Transiet Polymer Network Modelling
In self-healing materials, the crosslinks networking the polymers can dynamically break and re-form, i.e., transient bonds. Due to the dynamic features of the crosslinks, the transient network can exhibit interesting viscoelastic responses, and we are developing continuum theories to understand its rheological properties.
  • F. Meng*, M. Saed and E. Terentjev*, "Elasticity and relaxation in full and partial vitrimer networks." Macromolecules527423-7429 (2019).
  • J.-H. Chen, D.-D. Hu, Y.-D. Li, F. Meng*, J. Zhu, and J.-B. Zeng*, "Castor oil derived poly (urethane urea) networks with reprocessibility and enhanced mechanical properties." Polymer 143, 79-86 (2018). 
  • F. Meng, R. H. Pritchard, and E. Terentjev*, "Stress relaxation, dynamics and plasticity of transient polymer networks." Macromolecules 49,2843-2852 (2016). 
  • F. Meng, and E. Terentjev*, "Transient network at large deformations: elastic-plastic transition and necking instability." Polymers 8, 108 (2016). 
3. Drying Soft Matter Solutions
When soft matter solutions are being dried, there can be several sub-processes including solvent evaporation, solute diffusion, gel layer formation, etc. After drying process finishes, solutions can result in various forms such as coffee rings, solid particles, hollow particles, etc. We try to understand how different morphologies of soft matter solutions can evolve by constructing theoretical dynamic theories. 
  • F. Meng*, L. Luo, M. Doi* and Z-C. Ouyang, "Solute based Lagrangian scheme in modeling the drying process of soft matter solutions."European Physical Journal E 39, 22 (2016). 
  • L. Luo, F. Meng, J. Zhang, and M. Doi*, "Skin formation in drying a film of soft matter solutions -- application of solute based Lagrangian scheme." Chinese Physics B 25, 076801 (2016).
  • F. Meng, M. Doi*, and Z-C. Ouyang, "Cavitation in drying droplets of soft matter solutions."Physical Review Letters 113, 098301 (2014). 
4. Rubber/Gel Elasticity
Rubbers/gels are ubiquitous in our daily life, and in physics they are interesting in terms of their tunable mechanic properties. By utilizing the elastic theories, we can understand how and why rubber systems can behave under specific circumstances (for example, how to inflate a balloon in your childhood). 
  • F. Meng, J. Z. Y. Chen, M. Doi*, and Z-C. Ouyang, "Critical line in twisting instabilities of soft tubes." Soft Matter 11, 7046-7052 (2015). 
  • F. Meng, M. Doi, Z-C. Ouyang, X. Zheng, and P. Palffy-Muhoray*, "The 'coin-through-the rubber' trick: an elastically stabilized invagination." Journal of Elasticity 123, 43–57 (2015). 
  • F. Meng, J. Z. Y. Chen, M. Doi*, and Z-C. Ouyang, "Phase diagrams and interface in inflating balloon." AIChE Journal 60, 1393–1399 (2014). 
5. Polymer Composites
  • D. QianF. Meng*, "Modelling Mullins Effect Induced by Chain Delamination and Reattachment", Polymer, 222123608 (2021). 
  • H. S. Varol*, A. Srivastava, S. Kumar, M. Bonn, F. Meng, and S. H. Parekh*, "Bridging chains mediate nonlinear mechanics of polymer nanocomposites under cyclic deformation", Polymer 200, 122529 (2020). 
  • S. Varol, F. Meng, B. Hosseinkhani, C. Malm, D. Bonn, M. Bonn, A. Zaccone, and S. H. Parekh*, "Nanoparticle amount, and not size, determines chain alignment and nonlinear hardening in polymer nanocomposites." Proceedings of the National Academy of Sciences USA 114, E3170–E3177 (2017). 
6.Liquid-Liquid Phase Separation
Liquid-liquid phase transition is treated as connected to the formation of membraneless organelles in cells, and we try to construct a continuum theory for understanding the criterion of such transition and predicting the phase separated products in a liquid mixture constrained by an elastic network. 
  • X. Wei#, J. Zhou#, Y. Wang, and F. Meng*, "Modelling elastically mediated liquid-liquid phase separation",  Physical Review Letters, 125, 268001 (2020).